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A-Level Substitution and elimination in halogen compounds

What the A-Level syllabus expects for Substitution and elimination in halogen compounds, and how to practise it.

What the syllabus expects

How it's examined

Questions on this topic most often ask you to compare, explain. About 1% of the past-paper style questions in Rae's bank for this subject sit in this topic.

Worked examples

Example 1 (3 marks)

Phenylmethanol (C6H5CH2OH) may alternatively be made from methylbenzene in a two-step sequence. Propose a route for this synthesis, stating every reagent and condition needed.

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Step 1 (side-chain substitution): react methylbenzene, C6H5CH3, with chlorine, Cl2, in the presence of ultraviolet light (or heat). This free-radical substitution of a methyl hydrogen gives (chloromethyl)benzene, C6H5CH2Cl. Step 2 (hydrolysis): warm/reflux C6H5CH2Cl with aqueous sodium hydroxide, NaOH(aq). The halogen is replaced by OH, giving phenylmethanol, C6H5CH2OH.

Example 2 (2 marks)

Decide whether thiolates (R-S⁻) are more powerful nucleophiles than alkoxides (R-O⁻), and explain your reasoning.

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Compare nucleophilicity of R-S^- versus R-O^-. Sulfur sits below oxygen in Group 16, so it is a larger atom with more diffuse, polarisable valence electrons. The negative charge on the thiolate is spread over a larger volume, making S less tightly bound to its electrons than O. These loosely held, polarisable electrons are more readily distorted toward an electrophilic carbon, so thiolates form the new bond more easily. Sulfur is also less electronegative than oxygen, so it holds its lone pair less tightly and donates it more willingly. Therefore thiolates are the stronger (more powerful) nucleophiles.

Example 3 (2 marks)

Treating 2-nitrochlorobenzene with aqueous NaOH, and then adding a suitable acid, produces 2-nitrophenol. Draw the mechanism for this conversion.

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This is nucleophilic aromatic substitution (addition-elimination). Step 1: the hydroxide ion OH- attacks the ring carbon bearing the Cl atom; the resulting negative charge is delocalised onto the ortho -NO2 group (and the ring), giving a stabilised Meisenheimer-type intermediate. Step 2: the C-Cl bond breaks, expelling Cl- and restoring aromaticity to give the 2-nitrophenoxide ion. Adding acid then protonates the phenoxide to give 2-nitrophenol.

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More A-Level H2 Chemistry topics

The make-up of the atom and how its electrons are arranged · How atoms bond and how that governs a substance's behaviour · Ideal gases and working with gas mixtures · Competing definitions of acids and bases · Trends in the elements across a period and down a group · The mole and reacting-quantity calculations · all of A-Level H2 Chemistry